We don’t know why [stoppi71] needs to do gamma spectroscopy. We only know that he has made one, including a high-voltage power supply, a photomultiplier tube, and–what else–an Arduino. You also need a scintillation crystal to convert the gamma rays to visible light for the tube to pick up.
He started out using an open source multichannel analyzer (MCA) called Theremino. This connects through a sound card and runs on a PC. However, he wanted to roll his own and did so with some simple circuitry and an Arduino.